Understanding Battery Interfaces by Combined Characterizationand Simulation Approaches: Challenges and Perspectives
Understanding Battery Interfaces by Combined Characterizationand Simulation Approaches: Challenges and Perspectives
Driven by the continuous search for improving performances, understandingthe phenomena at the electrode/electrolyte interfaces has become an overridingfactor for the success of sustainable and efficient battery technologiesfor mobile and stationary applications. Toward this goal, rapid advances have...
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Personal Name(s): | Duncan, Atkins |
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Elixabete, Ayerbe / Benayad, Anass / Capone, Federico G. / Enio, Capria / Ivano, Casteli E. / Cekic-Laskovic, Isidora / Raul, Ciria / Dudy, Lenart / Edström, Kristina / Johnson, Mark R. / Li, Hongjiao / Lastra, Juan Maria Garcia / Souza, Matheus Leal De / Meunier, Valentin / Morcrette, Mathieu / Reichert, Harald / Simon, Patrice / Rueff, Jean-Pascal / Sottmann, Jonas / Wenzel, Wolfgang (Corresponding author) / Grimaud, Alexis (Corresponding author) | |
Contributing Institute: |
Helmholtz-Institut Münster Ionenleiter für Energiespeicher; IEK-12 |
Published in: | Advanced energy materials, 12 (2022) 17, S. 2102687 |
Imprint: |
Weinheim
Wiley-VCH
2022
|
DOI: |
10.1002/aenm.202102687 |
DOI: |
10.34734/FZJ-2023-05469 |
Document Type: |
Journal Article |
Research Program: |
BATTERY 2030+ large-scale research initiative: At the heart of a connected green society Battery Interface Genome - Materials Acceleration Platform Components and Cells |
Link: |
OpenAccess |
Publikationsportal JuSER |
Please use the identifier: http://dx.doi.org/10.34734/FZJ-2023-05469 in citations.
Driven by the continuous search for improving performances, understandingthe phenomena at the electrode/electrolyte interfaces has become an overridingfactor for the success of sustainable and efficient battery technologiesfor mobile and stationary applications. Toward this goal, rapid advances havebeen made regarding simulations/modeling techniques and characterizationapproaches, including high-throughput electrochemical measurementscoupled with spectroscopies. Focusing on Li-ion batteries, current developmentsare analyzed in the field as well as future challenges in order to gaina full description of interfacial processes across multiple length/timescales;from charge transfer to migration/diffusion properties and interphases formation,up to and including their stability over the entire battery lifetime. Forsuch complex and interrelated phenomena, developing a unified workflowintimately combining the ensemble of these techniques will be critical tounlocking their full investigative potential. For this paradigm shift in batterydesign to become reality, it necessitates the implementation of researchstandards and protocols, underlining the importance of a concerted approachacross the community. With this in mind, major collaborative initiatives gatheringcomplementary strengths and skills will be fundamental if societal andenvironmental imperatives in this domain are to be met. |